Search for: All records

Surface depletion field would introduce the depletion region near surface and thus could significantly alter the optical, electronic and optoelectronic properties of the materials, especially low-dimensional materials. Two-dimensional (2D) organic—inorganic hybrid perovskites with van der Waals bonds in the out-of-plane direction are expected to have less influence from the surface depletion field; nevertheless, studies on this remain elusive. Here we report on how the surface depletion field affects the structural phase transition, quantum confinement and Stark effect in 2D (BA)2PbI4 perovskite microplates by the thickness-, temperature- and power-dependent photoluminescence (PL) spectroscopy. Power dependent PL studies suggest that high-temperature phase (HTP) and low-temperature phase (LTP) can coexist in a wider temperature range depending on the thickness of the 2D perovskite microplates. With the decrease of the microplate thickness, the structural phase transition temperature first gradually decreases and then increases below 25 nm, in striking contrast to the conventional size dependent structural phase transition. Based on the thickness evolution of the emission peaks for both high-temperature phase and low-temperature phase, the anomalous size dependent phase transition could probably be ascribed to the surface depletion field and the surface energy difference between polymorphs. This explanation was further supported by the temperature dependent PL studies of the suspended microplates and encapsulated microplates with graphene and boron nitride flakes. Along with the thickness dependent phase transition, the emission energies of free excitons for both HTP and LTP with thickness can be ascribed to the surface depletion induced confinement and Stark effect. 

The existence of topological hinge states is a key signature for a newly proposed class of topological matter, the second-order topological insulators. In the present paper, a universal mechanism to generate chiral hinge states in the ferromagnetic axion insulator phase is introduced, which leads to an exotic transport phenomenon, the quantum anomalous Hall effect (QAHE) on some particular surfaces determined by both the crystalline symmetry and the magnetization direction. A realistic material system, Sm-doped Bi2Se3, is then proposed to realize such exotic hinge states by combining first-principles calculations and Green’s function techniques. A physically accessible way to manipulate the surface QAHE is also proposed, which makes it very different from the QAHE in ordinary 2D systems. 

As two of the five traditional human senses (sight, hearing, taste, smell, and touch), vision and sound are basic sources through which humans understand the world. Often correlated during natural events, these two modalities combine to jointly affect human perception. In this paper, we pose the task of generating sound given visual input. Such capabilities could help enable applications in virtual reality (generating sound for virtual scenes automatically) or provide additional accessibility to images or videos for people with visual impairments. As a first step in this direction, we apply learning-based methods to generate raw waveform samples given input video frames. We evaluate our models on a dataset of videos containing a variety of sounds (such as ambient sounds and sounds from people/animals). Our experiments show that the generated sounds are fairly realistic and have good temporal synchronization with the visual inputs.